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Thermal Stoner-Wohlfarth model for magnetodynamics of single domain nanoparticles

Autor(en)
Deniz Mostarac, Andrey A. Kuznetsov, Santiago Helbig, Claas Abert, Pedro A. Sánchez, Dieter Suess, Sofia S. Kantorovich
Abstrakt

We present the thermal Stoner-Wohlfarth (tSW) model and apply it in the context of molecular dynamics simulations. The model is validated against an ensemble of immobilized, randomly oriented uniaxial particles (solid superparamagnet) and a classical dilute ferrofluid for different combinations of anisotropy strength and magnetic field/moment coupling, at a fixed temperature. We compare analytical and simulation results to quantify the viability of the tSW model in reproducing the equilibrium properties (with and without dipole-dipole interactions) and dynamic properties (without dipole-dipole interactions) of magnetic soft matter systems. We show that if the anisotropy of a particle is more than five times higher than the thermal fluctuations, the tSW model is applicable and efficient. This approach allows one to consider the interplay between Néel and Brownian relaxation, often neglected in the fixed point-dipole representation-based magnetic soft matter theoretical investigations.

Organisation(en)
Computergestützte Physik und Physik der Weichen Materie, Physik Funktioneller Materialien
Externe Organisation(en)
Università degli Studi di Roma La Sapienza, Delft University of Technology
Journal
Physical Review B
Band
111
Anzahl der Seiten
14
ISSN
2469-9950
DOI
https://doi.org/10.48550/arXiv.2408.06136
Publikationsdatum
01-2025
Peer-reviewed
Ja
ÖFOS 2012
103043 Computational Physics, 103015 Kondensierte Materie
ASJC Scopus Sachgebiete
Electronic, Optical and Magnetic Materials, Condensed Matter Physics
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/e7233f47-48dd-4f7d-9424-2dd09b82dd8e