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Superconductivity in Ternary Mg<sub>4</sub>Pd<sub>7</sub>As<sub>6</sub>

Autor(en)
Hanna Świątek, Sylwia Gutowska, Michał J. Winiarski, Bartlomiej Wiendlocha, Tomasz Klimczuk
Abstrakt

The synthesis and characterization of a new compound Mg4Pd7As6, which is found to be a superconductor with Tc = 5.45 K is reported. Powder X-ray diffraction confirms the U4Re7Si6 structure (space group Im-3m, no. 229) with the lattice parameter a = 8.2572(1) Å. Magnetization, specific heat, and electrical resistivity measurements indicate that it is a moderate-coupling (λ = 0.72) type-II superconductor. The electronic and phonon structures are calculated, highlighting the importance of antibonding Pd–As interactions in determining the properties of this material. The calculated electron–phonon coupling parameter λ = 0.76 agrees very well with the experimental finding, which confirms the conventional pairing mechanism in Mg4Pd7As6.

Organisation(en)
Computergestützte Materialphysik
Externe Organisation(en)
Gdańsk University of Technology, AGH University of Science and Technology
Journal
Advanced Electronic Materials
Anzahl der Seiten
12
ISSN
2199-160X
DOI
https://doi.org/10.1002/aelm.202400284
Publikationsdatum
11-2024
Peer-reviewed
Ja
ÖFOS 2012
103033 Supraleitung, 103018 Materialphysik
Schlagwörter
ASJC Scopus Sachgebiete
Electronic, Optical and Magnetic Materials
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/397f5dbe-f932-403c-a5ea-85ee25e4421c